Ferrotoroidic ground state in a heterometallic {CrIIIDyIII6} complex displaying slow magnetic relaxation
Identifieur interne : 000C26 ( Main/Exploration ); précédent : 000C25; suivant : 000C27Ferrotoroidic ground state in a heterometallic {CrIIIDyIII6} complex displaying slow magnetic relaxation
Auteurs : Kuduva R. Vignesh [Inde] ; Alessandro Soncini ; Stuart K. Langley ; Wolfgang Wernsdorfer [Allemagne] ; Keith S. Murray ; Gopalan Rajaraman [Inde]Source :
- Nature Communications [ 2041-1723 ] ; 2017.
Abstract
Toroidal quantum states are most promising for building quantum computing and information storage devices, as they are insensitive to homogeneous magnetic fields, but interact with charge and spin currents, allowing this moment to be manipulated purely by electrical means. Coupling molecular toroids into larger toroidal moments via ferrotoroidic interactions can be pivotal not only to enhance ground state toroidicity, but also to develop materials displaying ferrotoroidic ordered phases, which sustain linear magneto–electric coupling and multiferroic behavior. However, engineering ferrotoroidic coupling is known to be a challenging task. Here we have isolated a {CrIIIDyIII6} complex that exhibits the much sought-after ferrotoroidic ground state with an enhanced toroidal moment, solely arising from intramolecular dipolar interactions. Moreover, a theoretical analysis of the observed sub-Kelvin zero-field hysteretic spin dynamics of {CrIIIDyIII6} reveals the pivotal role played by ferrotoroidic states in slowing down the magnetic relaxation, in spite of large calculated single-ion quantum tunneling rates.
Url:
DOI: 10.1038/s41467-017-01102-5
PubMed: 29044098
PubMed Central: 5647347
Affiliations:
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Murray</name><affiliation><nlm:aff id="Aff5"><institution-wrap><institution-id institution-id-type="ISNI">0000 0004 1936 7857</institution-id><institution-id institution-id-type="GRID">grid.1002.3</institution-id><institution>School of Chemistry, Monash University,</institution></institution-wrap>Melbourne, VIC 3800 Australia</nlm:aff><wicri:noCountry code="subfield">VIC 3800 Australia</wicri:noCountry></affiliation></author><author><name sortKey="Rajaraman, Gopalan" sort="Rajaraman, Gopalan" uniqKey="Rajaraman G" first="Gopalan" last="Rajaraman">Gopalan Rajaraman</name><affiliation wicri:level="1"><nlm:aff id="Aff6"><institution-wrap><institution-id institution-id-type="ISNI">0000 0001 2198 7527</institution-id><institution-id institution-id-type="GRID">grid.417971.d</institution-id><institution>Department of Chemistry,</institution><institution>Indian Institute of Technology Bombay,</institution></institution-wrap>Mumbai, 400076 India</nlm:aff><country xml:lang="fr">Inde</country><wicri:regionArea>Mumbai</wicri:regionArea></affiliation></author></analytic><series><title level="j">Nature Communications</title><idno type="eISSN">2041-1723</idno><imprint><date when="2017">2017</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p id="Par1">Toroidal quantum states are most promising for building quantum computing and information storage devices, as they are insensitive to homogeneous magnetic fields, but interact with charge and spin currents, allowing this moment to be manipulated purely by electrical means. Coupling molecular toroids into larger toroidal moments via ferrotoroidic interactions can be pivotal not only to enhance ground state toroidicity, but also to develop materials displaying ferrotoroidic ordered phases, which sustain linear magneto–electric coupling and multiferroic behavior. However, engineering ferrotoroidic coupling is known to be a challenging task. Here we have isolated a {Cr<sup>III</sup>Dy<sup>III</sup><sub>6</sub>} complex that exhibits the much sought-after ferrotoroidic ground state with an enhanced toroidal moment, solely arising from intramolecular dipolar interactions. Moreover, a theoretical analysis of the observed sub-Kelvin zero-field hysteretic spin dynamics of {Cr<sup>III</sup>Dy<sup>III</sup><sub>6</sub>} reveals the pivotal role played by ferrotoroidic states in slowing down the magnetic relaxation, in spite of large calculated single-ion quantum tunneling rates.</p></div></front><back><div1 type="bibliography"><listBibl><biblStruct><analytic><author><name sortKey="Christou, G" uniqKey="Christou G">G Christou</name></author><author><name sortKey="Gatteschi, D" uniqKey="Gatteschi D">D Gatteschi</name></author><author><name sortKey="Hendrickson, Dn" uniqKey="Hendrickson D">DN Hendrickson</name></author><author><name sortKey="Sessoli, R" uniqKey="Sessoli R">R Sessoli</name></author></analytic></biblStruct><biblStruct></biblStruct><biblStruct><analytic><author><name sortKey="Gatteschi, D" uniqKey="Gatteschi D">D Gatteschi</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Gatteschi, D" uniqKey="Gatteschi D">D 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W">WR Wadt</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Cundari, Tr" uniqKey="Cundari T">TR Cundari</name></author><author><name sortKey="Stevens, Wj" uniqKey="Stevens W">WJ Stevens</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Noodleman, L" uniqKey="Noodleman L">L Noodleman</name></author></analytic></biblStruct><biblStruct></biblStruct><biblStruct><analytic><author><name sortKey="Rousochatzakis, I" uniqKey="Rousochatzakis I">I Rousochatzakis</name></author><author><name sortKey="Luban, M" uniqKey="Luban M">M Luban</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Leuenberger, Mn" uniqKey="Leuenberger M">MN Leuenberger</name></author><author><name sortKey="Loss, D" uniqKey="Loss D">D Loss</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Lascialfari, A" uniqKey="Lascialfari A">A Lascialfari</name></author><author><name sortKey="Jang, Zh" uniqKey="Jang Z">ZH Jang</name></author><author><name sortKey="Borsa, F" uniqKey="Borsa F">F Borsa</name></author><author><name sortKey="Carretta, P" uniqKey="Carretta P">P Carretta</name></author><author><name sortKey="Gatteschi, D" uniqKey="Gatteschi D">D Gatteschi</name></author></analytic></biblStruct></listBibl></div1></back></TEI><affiliations><list><country><li>Allemagne</li><li>Inde</li></country></list><tree><noCountry><name sortKey="Langley, Stuart K" sort="Langley, Stuart K" uniqKey="Langley S" first="Stuart K." last="Langley">Stuart K. Langley</name><name sortKey="Murray, Keith S" sort="Murray, Keith S" uniqKey="Murray K" first="Keith S." last="Murray">Keith S. Murray</name><name sortKey="Soncini, Alessandro" sort="Soncini, Alessandro" uniqKey="Soncini A" first="Alessandro" last="Soncini">Alessandro Soncini</name></noCountry><country name="Inde"><noRegion><name sortKey="Vignesh, Kuduva R" sort="Vignesh, Kuduva R" uniqKey="Vignesh K" first="Kuduva R." last="Vignesh">Kuduva R. Vignesh</name></noRegion><name sortKey="Rajaraman, Gopalan" sort="Rajaraman, Gopalan" uniqKey="Rajaraman G" first="Gopalan" last="Rajaraman">Gopalan Rajaraman</name></country><country name="Allemagne"><noRegion><name sortKey="Wernsdorfer, Wolfgang" sort="Wernsdorfer, Wolfgang" uniqKey="Wernsdorfer W" first="Wolfgang" last="Wernsdorfer">Wolfgang Wernsdorfer</name></noRegion></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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